Gábor, M., Tóth, M., Kristóf, M., Komáromi-Hiller,
G., (1995): Thermal behavior and decomposition of intercalated kaolinite.
Clays and Clay
Minerals, 43. 2. 223-228.
Abstract:
Intercalation complexes of a Hungarian kaolinite were prepared with
hydrazine and potassium acetate. The thermal behavior and decomposition
of the kaolinite-potassium acetate complex was studied by simultaneous
TA-EGA, XRD, and FTIR methods. The intercalation complex is stable up to
300 degrees C, and decomposition takes place in two stages after melting
of potassium acetate intercalated in the interlayer spaces. Dehydroxylation
occurred, in the presence of a molten phase, at a lower temperature than
for the pure kaolinite. FTIR studies revealed that there is a sequence
of dehydroxylation for the various OH groups of intercalated kaolinite.
The reaction mechanism was followed up to 1000 degrees C via identification
of the gaseous and solid decomposition products formed: H2O, CO2, CO, C3H6O,
intercalated phases with basal spacings of 14.1 Angstrom, 11.5 Angstrom,
and 8.5 Angstrom as well as elemental carbon, K4H2(CO3)(3) . 1.5H(2)O,
K2CO3 . 1.5H(2)O, and KAlSiO4.
Author Keywords:
INFRARED SPECTROSCOPY, INTERCALATION, KAOLINITE, THERMAL ANALYSIS,
X-RAY POWDER DIFFRACTION